As Smugglers owners, we have spent 20 weeks there since 1997.
We drive around a lot and have always looked for moose in any boggy areas we pass, where they typically are supposed to be. Also just look, in general..
Have only seen one, once, and that was on the Mountain Road between Stowe and Smugglers. We saw a line of cars stopped and some people were out of their cars, looking into the woods, so we did too and were rewarded with a moose.
Although there are many in the state, they are not that easy to spot, apparently. Enjoy Vermont and the area.
Good luck!